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Chronicle of Philanthropy - Data
"Provides links to surveys conducted by The Chronicle of Philanthropy and to Chronicle articles that report on studies on philanthropy that are conducted by other organizations."
National Center for Charitable Statistics
This is "the national clearinghouse of data on the nonprofit sector in the United States."
County Level Data Sets
From the USDA - ERS, this site provides state and county-level data on population, poverty, education, employment, unemployment, and median household income.